光学学报, 2016, 36 (4): 0401001, 网络出版: 2016-04-05
华北平原污染气体区域分布的车载DOAS 遥测研究
Study on Regional Distribution of Air Pollutants in North China Plain by Mobile DOAS
大气光学 车载差分光学吸收光谱技术 垂直柱浓度 华北平原 atmospheric optics mobile differential optical absorption spectroscop vertical column density North China Plain SO2 SO2 NO2 NO2
摘要
利用车载差分光学吸收光谱技术(DOAS)于2013 年6 月至7 月对华北平原进行走航观测,研究了不同风场下SO2和NO2的柱浓度空间分布特征及其对北京地区的影响。研究发现,在石家庄、保定和济南附近同时观测到SO2和NO2 高值,表明三地附近存在工业排放源,其中6 月11 日石家庄附近观测到SO2 和NO2高值区域均值分别为1.29×1017 molecule·cm-2和3.59×1016 molecule·cm-2,为低值区域均值的3.8倍和3.6倍。在西南稳定风场下,石家庄—保定—北京方向为一条污染物输送通道,Hysplit 风场轨迹模型结果也验证了该输送通道的存在。车载DOAS 观测的NO2 柱浓度和臭氧检测仪(OMI)检测结果的对比显示,两者具有较好的一致性;同时卫星观测也验证了偏南风场下污染物输送通道的存在。实验结果表明车载DOAS 技术在污染物排放源监测、空气污染物地区分布快速获取以及卫星数据校验方面都具有重要作用。
Abstract
Mobile differential optical absorption spectroscopy (DOAS) is used to study regional distribution of SO2 and NO2 column density in the North China Plain and its impact on the Beijing region under different wind fields during June and July in 2013. High SO2 and NO2 concentration values around Shijiazhuang, Baoding and Jinan areas are observed simultaneously, indicating that there are industrial emission sources in these areas. Average values of SO2 and NO2 around the Shijiazhuang area on June 11th are 1.29×1017 molecule·cm-2 and 3.59× 1016 molecule · cm- 2, respectively, which are 3.8 times and 3.6 times of the average in low concentration area respectively. Shijiazhuang- Baoding- Beijing direction can be a transportation pathway in steady south- west wind field, and the conclusion is verified by the Hysplit model. NO2 column density obtained by mobile DOAS is compared with that by ozone monitoring instrument(OMI), and the good agreement is found. The satellite observation also proves existence of the transportation pathway in south wind field. The experimental results show that mobile DOAS plays an important role in detecting emission sources, rapidly obtaining regional distribution of air pollutants and validating satellite data.
牟福生, 李昂, 谢品华, 吴丰成, 张杰, 王杨. 华北平原污染气体区域分布的车载DOAS 遥测研究[J]. 光学学报, 2016, 36(4): 0401001. Mou Fusheng, Li Ang, Xie Pinhua, Wu Fengcheng, Zhang Jie, Wang Yang. Study on Regional Distribution of Air Pollutants in North China Plain by Mobile DOAS[J]. Acta Optica Sinica, 2016, 36(4): 0401001.