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Radiation-pressure-induced photoluminescence enhancement of all-inorganic perovskite CsPbBr3 quantum dots

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Abstract

Perovskite quantum dots (QDs) are of great interest due to their outstanding optoelectronic properties and tremendous application potential. Improving photoluminescence (PL) spectra in all-inorganic perovskite QDs is of great importance for performance enhancement. In this work, the PL quantum yield of the CsPbBr3 perovskite QDs is enhanced from 70% to 95% with increasing radiation pressure. Such enhancement is attributed to the increased binding energy of self-trapped excitons (STEs) upon radiation pressure, which is consistent with its blue-shifted PL and other characterization results. Furthermore, we study ultrafast absorption spectroscopy and find that the dynamics of relaxation from free excitons to STEs in radiation pressure CsPbBr3 QDs is ascribed to stronger electron–phonon coupling in the contracted octahedral structure. It is further demonstrated that radiation pressure can boost the PL efficiency and explore effectively the relationship between the structure and optical properties.

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DOI:10.1364/PRJ.7.000837

所属栏目:Optical and Photonic Materials

基金项目:National Key RD Program of China; China Postdoctoral Science Foundation10.13039/501100002858; Natural Science Foundation of Guangdong Province10.13039/501100003453; National Natural Science Foundation of China (NSFC)10.13039/501100001809; Science Technology Innovation Committee Foundation of Shenzhen;

收稿日期:2019-03-12

录用日期:2019-05-26

网络出版日期:2019-07-11

作者单位    点击查看

Ying Zhang:Center for Advanced Material Diagnostic Technology, College of Engineering Physics, Shenzhen Technology University, Shenzhen 518118, ChinaGuangdong Provincial Key Laboratory of Mico/Nano Optomechatronics Engineering, College of Optoelectronic Engineering, Shenzhen University, Shenzhen 518060, China
Haiou Zhu:College of New Materials and New Energies, Shenzhen University of Technology, Shenzhen 518118, China
Taiwu Huang:Center for Advanced Material Diagnostic Technology, College of Engineering Physics, Shenzhen Technology University, Shenzhen 518118, China
Zongpeng Song:Guangdong Provincial Key Laboratory of Mico/Nano Optomechatronics Engineering, College of Optoelectronic Engineering, Shenzhen University, Shenzhen 518060, China
Shuangchen Ruan:Guangdong Provincial Key Laboratory of Mico/Nano Optomechatronics Engineering, College of Optoelectronic Engineering, Shenzhen University, Shenzhen 518060, ChinaCollege of New Materials and New Energies, Shenzhen University of Technology, Shenzhen 518118, China

联系人作者:Shuangchen Ruan(scruan@szu.edu.cn)

备注:National Key RD Program of China; China Postdoctoral Science Foundation10.13039/501100002858; Natural Science Foundation of Guangdong Province10.13039/501100003453; National Natural Science Foundation of China (NSFC)10.13039/501100001809; Science Technology Innovation Committee Foundation of Shenzhen;

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引用该论文

Ying Zhang, Haiou Zhu, Taiwu Huang, Zongpeng Song, and Shuangchen Ruan, "Radiation-pressure-induced photoluminescence enhancement of all-inorganic perovskite CsPbBr3 quantum dots," Photonics Research 7(8), 837-846 (2019)

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