中国激光, 2014, 41 (10): 1014003, 网络出版: 2014-08-26   

差分吸收激光雷达监测北京灰霾天臭氧时空分布特征 下载: 515次

Temporal and Spatial Distribution Characteristics of Ozone Based on Differential Absorption Lidar in Beijing
作者单位
中国科学院安徽光学精密机械研究所大气成分与光学重点实验室, 安徽 合肥 230031
摘要
差分吸收激光雷达是测量对流层臭氧时空分布的有力工具,利用差分吸收激光雷达在灰霾条件下开展观测研究,分析了臭氧浓度时空分布特征。结果表明:在夏季副热带高压大气天气条件下,受偏南风气团输送的影响,6月中旬形成一次高浓度的臭氧污染过程。6月14日夜间至6月15日中午离地面1.5~2 km高度的臭氧气团浓度(即体积分数)高达1.2×10-7以上,下午臭氧气团出现下沉,从而引起当日下午近地面臭氧浓度的升高。在灰霾天气过程中,细颗粒物与臭氧分布在不同高度上具有不同的关联特征,地面颗粒物充分参与了光化学反应过程,而高空高浓度的颗粒物和臭氧气体则与输送有关。晴朗天气下的臭氧浓度在整个空间尺度上都有不同程度的下降,并且没有出现明显的外部输入气团。
Abstract
The differential absorption lidar is an effective tool for measuring ozone distributions. In the haze event, the differential absorption lidar is carried out to observe the temporal and spatial distribution characteristics of ozone concentration. The results show that a high ozone pollution process is caused by southwest airflow together with the influence of subtropical anticyclone in mid June. From the night of June 14 to midday of June 15, ozone concentration in high altitude reaches above 1.2×10-7. And the ozone gas ranging from 1.5 km to 2 km moves down to the surface, thus causing the increase of surface ozone concentration afternoon on June 15. In the haze period, the distributions of fine particulates and ozone show different characteristics in different heights. Specifically the near-ground particles completely participate in the photochemical reaction process, while particles and ozone with are more related to transportation. In addition ozone concentration in clear weather is low and no obvious external input air mass is observed.

范广强, 张天舒, 付毅宾, 董云升, 陈臻懿, 刘建国, 刘文清. 差分吸收激光雷达监测北京灰霾天臭氧时空分布特征[J]. 中国激光, 2014, 41(10): 1014003. Fan Guangqiang, Zhang Tianshu, Fu Yibin, Dong Yunsheng, Chen Zhenyi, Liu Jianguo, Liu Wenqing. Temporal and Spatial Distribution Characteristics of Ozone Based on Differential Absorption Lidar in Beijing[J]. Chinese Journal of Lasers, 2014, 41(10): 1014003.

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