用计算量子场论方法研究了非线性啁啾频率对势阱中正负电子对产生的增强效应。研究了由静态势阱和动态势阱组成的组合势阱中产生的正负电子对的密度、产额和能谱等性质随着啁啾参数的变化，分析了组合势阱的频谱和瞬时束缚态。发现非线性啁啾效应对低频区域比较敏感，与固定频率情况相比可以使粒子数增加2～3倍。与组合势阱相比，非线性啁啾效应对单个振荡势阱更敏感。在低频下单个振荡的势阱中正负电子对产额可提高多个数量级。这是因为在低频下单个振荡的势阱中，主要通过量子隧穿过程产生的正负电子对数目非常低。非线性啁啾效应增加了高频场成分，提高了多光子过程和动力学辅助机制。由于高频抑制作用，所以非线性啁啾效应对高频区域粒子的增量不大，甚至会抑制正负电子对的产生。

We investigate femtosecond laser trapping dynamics of two-photon absorbing hollow-core nanoparticles with different volume fractions and two-photon absorption (TPA) coefficients. Numerical simulations show that the hollow-core particles with low and high-volume fractions can easily be trapped and bounced by the tightly focused Gaussian laser pulses, respectively. Further studies show that the hollow-core particles with and without TPA can be identified, because the TPA effect enhances the radiation force, and subsequently the longitudinal force destabilizes the trap by pushing the particle away from the focal point. The results may find direct applications in particle sorting and characterizing the TPA coefficient of single nanoparticles.

Mechanical exfoliation (ME) and chemical vapor deposition (CVD) MoS₂ monolayers have been extensively studied, but the large differences of nonlinear optical performance between them have never been clarified. Here, we prepared MoS₂ monolayers using ME and CVD methods and investigated the two-photon absorption (TPA) response and its saturation. We found that the TPA coefficient of the ME monolayer was about (1.88 ± 0.21) × 10³ cm/GW, nearly two times that of the CVD one at (1.04 ± 0.15) × 10³ cm/GW. Furthermore, we simulated and compared the TPA-induced optical pulse modulation in multilayer cascaded structures, which is instructive and meaningful for the design of optical devices such as a beam shaper and optical limiter.

Laser-induced modification at 355 nm of deuterated potassium dihydrogen phosphate (DKDP) crystals following exposure to nanosecond (ns) and sub-ns laser irradiation is investigated in order to probe the absorption mechanism in damage initiation. Laser damage resistance is greatly improved by sub-ns laser conditioning, whereas only a little improvement occurred after ns laser conditioning at the same laser fluence. Moreover, scattering and transmittance variations after the two types of laser conditioning indicate similar reduction of linear absorption. However, by contrast, large differences on nonlinear absorption modification are discovered using Z-scan measurement. This characteristic absorption modification by laser irradiation provides evidence that a nonlinear absorption mechanism plays a key role in damage initiation at 355 nm.

The nonlinear absorption (NLA) properties of potassium dideuterium phosphate crystals at 515 nm under different excitation laser intensities are investigated with the Z-scan technique. Two critical intensities are highlighted: the critical intensity for exciting the NLA and the critical intensity of the multiphoton absorption mechanism transition. Experimental results indicate the existence of defect states located in the band gap, which can be manipulated by varying laser intensity. A model based on the change of multiphoton absorption mechanism induced by the transformation of defect species is proposed to interpret the experiments. Modeling results are in good agreement with the experiment data.

Using the classical-trajectory Monte Carlo model, we have theoretically studied the angular momentum distribution of frustrated tunneling ionization (FTI) of atoms in strong laser fields. Our results show that the angular momentum distribution of the FTI events exhibits a double-hump structure. With this classical model, we back traced the tunneling coordinates, i.e., the tunneling time and initial transverse momentum at tunneling ionization. It is shown that for the events tunneling ionized at the rising edge of the electric field, the final angular momentum exhibits a strong dependence on the initial transverse momentum at tunneling. While for the events ionized at the falling edge, there is a relatively harder recollision between the returning electron and the parent ion, leading to the angular momentum losing the correlation with the initial transverse momentum. Our study suggests that the angular momentum of the FTI events could be manipulated by controlling the initial coordinates of the tunneling ionization.

Photoassociation via reverse ladder transition controlled by two and four laser pulses is investigated using the time-dependent quantum wave packet method. The calculated results show that the amplitudes of the pulses have an enormous effect on the target population and total yield of association. For the target state with a high energy level, the population of background states can reduce the state-selectivity. Although, the total yield of association is decreased, the four pulses can induce the population transferring to low vibrational levels, and the state-selectivity of the target state is high.

We investigate the superposition properties of the dipole and quadrupole plasmon modes in the near field both experimentally, by using photoemission electron microscopy (PEEM), and theoretically. In particular, the asymmetric near-field distributions on gold (Au) nanodisks and nanoblocks under oblique incidence with different polarizations are investigated in detail. The results of PEEM measurements show that the evolutions of the asymmetric near-field distributions are different between the excitation with s-polarized and p-polarized light. The experimental results can be reproduced very well by numerical simulations and interpreted as the superposition of the dipole and quadrupole modes with the help of analytic calculations. Moreover, we hypothesize that the electrons collected by PEEM are mainly from the plasmonic hot spots located at the plane in the interface between the Au particles and the substrate in the PEEM experiments.

A 1470 nm+852 nm two-color (TC) cesium (Cs) magneto-optical trap (MOT) with a 6S1/2-6P3/2-7S1/2 ladder-type system is proposed and experimentally investigated. To the best of our knowledge, it is the first report about the 1470 nm+852 nm Cs TC-MOT. One of the three pairs of the 852 nm cooling and trapping beams (CTBs) in a conventional Cs MOT is replaced with a pair of the 1470 nm CTBs. Thus, the TC-MOT partially employs the optical radiation forces from photon scattering of the 6P3/2 (F′=5) 7S1/2 (F′′=4) excited-state transition (1470 nm). This TC-MOT can cool and trap Cs atoms on both the red- and blue-detuning sides of the two-photon resonance. This work may have applications in cooling and trapping of atoms using inconvenient wavelengths and background-free detection of cold and trapped Cs atoms.