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被动多轴差分吸收光谱技术监测大气NO2垂直廓线研究

Retrieval of Atmospheric NO2 Vertical Profile from Multi-Axis Differential Optical Absorption Spectroscopy

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摘要

痕量气体垂直廓线的监测,对大气污染研究具有重要意义。介绍了被动多轴差分吸收光谱(MAX-DOAS)技术监测痕量气体垂直廓线的光学遥感方法。研究中MAX-DOAS测量多个角度的斜柱浓度、结合大气辐射传输模型,利用最优估算法反演出痕量气体垂直廓线,并对最优估算法参数选取和反演评估进行了详细描述。将该技术应用于合肥地区NO2垂直廓线的监测:通过与长光程差分吸收光谱仪的测量结果对比,相关系数达到0.80。该技术为大气环境立体监测提供了一种简便的方法。

Abstract

Measurement of trace-gas vertical profile is very important for research of atmospheric pollution. The multi-axis differential optical absorption spectroscopy (MAX-DOAS) is used on trace-gas profile monitoring. Combing with radiative transfer models, trace gas vertical profile is derived from slant column densities of several elevation angles of MAX-DOAS with optimal estimation method. The parameters setup of retrieval algorithm and the characterization of the retrieval has been described in detail. MAX-DOAS is used to monitor NO2 profile of Hefei area. The measurement result is validated with long-path differential optical absorption spectroscopy (LP-DOAS), and the correlation coefficient is 0.80. This technique provides a simple and convenient method three-dimensional observation for air pollution.

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中图分类号:O433.4

DOI:10.3788/aos201131.1101007

所属栏目:大气与海洋光学

责任编辑:谢婧  信息反馈

基金项目:国家自然科学基金(40805015)和安徽省优秀青年科技基金(10040606Y28)资助课题。

收稿日期:2011-05-10

修改稿日期:2011-06-21

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周海金:中国科学技术大学精密机械与精密仪器系, 安徽 合肥 230026中国科学院安徽光学精密机械研究所环境光学与技术重点实验室, 安徽 合肥 230031
刘文清:中国科学院安徽光学精密机械研究所环境光学与技术重点实验室, 安徽 合肥 230031
司福祺:中国科学院安徽光学精密机械研究所环境光学与技术重点实验室, 安徽 合肥 230031
谢品华:中国科学院安徽光学精密机械研究所环境光学与技术重点实验室, 安徽 合肥 230031
徐晋:中国科学院安徽光学精密机械研究所环境光学与技术重点实验室, 安徽 合肥 230031
窦科:中国科学院安徽光学精密机械研究所环境光学与技术重点实验室, 安徽 合肥 230031

联系人作者:周海金(hjzhou@aiofm.ac.cn)

备注:周海金(1986—),男,博士研究生,主要从事差分吸收光谱技术方面的研究。

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引用该论文

Zhou Haijin,Liu Wenqing,Si Fuqi,Xie Pinhua,Xu Jin,Dou Ke. Retrieval of Atmospheric NO2 Vertical Profile from Multi-Axis Differential Optical Absorption Spectroscopy[J]. Acta Optica Sinica, 2011, 31(11): 1101007

周海金,刘文清,司福祺,谢品华,徐晋,窦科. 被动多轴差分吸收光谱技术监测大气NO2垂直廓线研究[J]. 光学学报, 2011, 31(11): 1101007

被引情况

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【5】刘进,司福祺,周海金,赵敏杰,窦科,刘文清. 被动差分吸收光谱技术测量大气中水汽垂直柱浓度. 光学学报, 2013, 33(8): 801002--1

【6】刘进,司福祺,周海金,赵敏杰,窦科,王煜,刘文清. 基于成像差分吸收光谱技术测量电厂SO2排放方法研究. 光学学报, 2015, 35(6): 630003--1

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