Fifth harmonic generation (5th HG) of a Nd:glass laser is an effective way to acquire high-energy coherent deep-ultraviolet radiation near 200 nm. In this work, cascade generation of the fifth harmonic of a Nd:glass laser in a 5 mm ammonium dihydrogen phosphate (ADP) crystal was investigated, and maximum conversion efficiency of 14% and large angular acceptance of 45 mrad were demonstrated at a noncritical phase-matching temperature of 75.1°C. However, as the results reveal, the temperature sensitivity and nonlinear absorption would hinder its high-energy application. As for that, based on the complementary relationship of the angle and temperature in the phase-matching condition, an upgraded focusing 5th HG design coupled with the cylindrical temperature distribution scheme was proposed. By this upgraded focusing design, more than the improvement of the conversion efficiency, the output 5ω near-field intensity distribution turns out to be insensitive to the temperature gradient. Potentially, this idea can be applied for many other frequency conversion schemes such as high-repetition frequency lasers, which have similar temperature gradient problems.

We present an Er-doped fiber (Er:fiber)-based femtosecond laser at 780 nm with 256 MHz repetition rate, 191 fs pulse duration, and over 1 W average power. Apart from the careful third-order dispersion management, we introduce moderate self-phase modulation to broaden the output spectrum of the Er:fiber amplifier and achieve 193 fs pulse duration and 2.43 W average power. Over 40% frequency doubling efficiency is obtained by a periodically poled lithium niobate crystal. Delivering through a hollow-core photonic bandgap fiber, this robust laser becomes an ideal and convenient light source for two-photon autofluorescence imaging.

An external frequency doubling electro-optically Q-switched neodymium-doped yttrium aluminum garnet (Nd:YAG) 473 nm blue laser was demonstrated. With absorbed pump energy of 48 mJ at 100 Hz repetition rate, about 2 mJ of 473 nm blue laser pulse energy was achieved by cascade frequency doubling. The second harmonic conversion efficiency was 64.5%, and overall optical-optical efficiency was 4.2%, respectively. The blue laser pulse width was less than 10 ns, and beam quality factor was less than 2.4.

A scheme for measuring the intra-cavity round-trip loss of an all-solid-state single-frequency laser by inserting a type-I noncritical phase-matching nonlinear crystal introducing nonlinear loss into the resonator is presented. The intra-cavity round-trip loss is theoretically deduced by analyzing the dependence of the fundamental-wave (FW) and second-harmonic-wave (SHW) powers on the pump factor and the nonlinear conversion factor of the single-frequency laser and experimentally measuring them by recording different FW and SHW powers, which are decided by the temperature of the nonlinear crystal. The measured intra-cavity round-trip loss and pump factor are 4.84% and 6.91% W 1, respectively. The standard deviations of the measured intra-cavity round-trip loss and the pump factor are 0.26% and 0.07%, respectively. This scheme is very suitable for measuring the intra-cavity round-trip loss of a high-gain solid-state single-frequency laser.

A high power continuous-wave single-frequency green fiber laser by second-harmonic generation of a Yb-doped fiber amplifier (YDFA) is developed. A linearly polarized single-mode fiber amplifier produces a 60 W infrared laser at 1064 nm with a 103 W incident diode pump laser at 976 nm, corresponding to an optical conversion efficiency of 58%. An external bow-tie enhancement cavity incorporating a noncritically phase-matched lithium triborate crystal is employed for second-harmonic generation. A 33.2 W laser at 532 nm is obtained with a 45 W incident 1064 nm fundamental laser, corresponding to a conversion efficiency of 74%.

A stable three-channel dual-wavelength fiber ring laser is proposed and experimentally demonstrated. The digital micromirror-device (DMD) processor can select and recirculate any dual waveband from the gain spectrum of the erbium-doped fiber at each channel. The uniform and stable dual-wavelength oscillation is obtained by a highly nonlinear photonic crystal fiber, which causes two degenerate the four-wave-mixing processes. By loading different reproducibility diffraction gratings on the optoelectronic DMD processor, the laser can be operated stably in a three-channel dual-wavelength scheme at room temperature. The power fluctuation of each laser channel is less than ～0.02 dB.